Optimizing Catalyst Performance: A Study of Support Addition Effects on La-Ni-Mn in Catalytic Dry Reforming of Methane
DOI:
https://doi.org/10.30572/2018/KJE/160405Keywords:
Methane dry reforming, Lanthanum-Nickel-Based Catalyst, Titanium, MCM-41, Perovskite, Catalyst activity, HydrogenAbstract
In this work, the effect of the support addition to LaNiMnO3 perovskite catalyst is investigated. Perovskite catalysts are prepared via the sol-gel method, namely LaNiMnO3 (LNMO3), LaNiMnO3/MCM-41 (LNMO3/MCM-41), and LaNiMnO3/TiO2 (LNMO3/TiO2). The catalysts are characterized using BET, TGA, XRD, FE-SEM, EDS, and FTIR techniques. The catalytic performances of those catalysts are evaluated in the catalytic dry reforming of methane to produce synthesis gas (H2 and CO). The results of this study indicate that the LNMO3/MCM-41 presents the highest rates of conversion for CH4 and CO2, with 80.56 and 76.32%, respectively. The optimal temperature of reaction to obtain the highest conversion of syngas is 800 °C. The order of activity and stability can be presented as LNMO3/MCM-41> LNMO3/TiO2 >LNMO3. To conclude, this research develops new catalysts with high catalytic performance to improve syngas production from the reaction of methane with carbon dioxide
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